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Photoelectrochemical asymmetric catalysis enables site- and enantioselective cyanation of benzylic C–H bonds - Nature Catalysis
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The enantioselective functionalization of ubiquitous C(sp3)–H bonds is ideally suited for the construction of three-dimensional chiral structures. However, organic molecules often contain multiple C(sp3)–H bonds with a similar energy and steric environment, rendering the simultaneous control of site-, chemo- and stereoselectivity extremely challenging.
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