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Directing CO2 electroreduction pathways for selective C2 product formation using single-site doped copper catalysts - Nature Chemical Engineering

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Directing CO2 electroreduction pathways for selective C2 product formation using single-site doped copper catalysts - Nature Chemical Engineering

Manipulating the selectivity-determining step in post-C–C coupling is crucial for enhancing C2 product specificity during electrocatalytic CO2 reduction, complementing efforts to boost rate-determining step kinetics. Here we highlight the role of single-site noble metal dopants on Cu surfaces in influencing C–O bond dissociation in an oxygen-bound selectivity-determining intermediate, steering post-C–C coupling toward ethylene versus ethanol.

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Directing CO2 electroreduction pathways for selective C2 product formation using single-site doped copper catalysts - Nature Chemical Engineering

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Directing CO2 electroreduction pathways for selective C2 product formation using single-site doped copper catalysts - Nature Chemical Engineering

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