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Ultrafast electronic relaxation pathways of the molecular photoswitch quadricyclane - Nature Chemistry

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Ultrafast electronic relaxation pathways of the molecular photoswitch quadricyclane - Nature Chemistry

The light-induced ultrafast switching between molecular isomers norbornadiene and quadricyclane can reversibly store and release a substantial amount of chemical energy. Prior work observed signatures of ultrafast molecular dynamics in both isomers upon ultraviolet excitation but could not follow the electronic relaxation all the way back to the ground state experimentally.

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Ultrafast electronic relaxation pathways of the molecular photoswitch quadricyclane - Nature Chemistry

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Ultrafast electronic relaxation pathways of the molecular photoswitch quadricyclane - Nature Chemistry

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