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Photoelectrochemical asymmetric dehydrogenative [2 + 2] cycloaddition between C–C single and double bonds via the activation of two C(sp3)–H bonds - Nature Catalysis
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The efficient generation of high structural complexity, which correlates with the number of stereocentres, is an important objective in organic synthesis. Ideally, from a perspective of economy and sustainability, the conversion should include the direct functionalization of unactivated C(sp3)–H bonds.
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