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Interplay between copper redox and transfer and support acidity and topology in low temperature NH3-SCR - Nature Communications

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Interplay between copper redox and transfer and support acidity and topology in low temperature NH3-SCR - Nature Communications

Low-temperature standard NH3-SCR over copper-exchanged zeolite catalysts occurs on NH3-solvated Cu-ion active sites in a quasi-homogeneous manner. As key kinetically relevant reaction steps, the reaction intermediate CuII(NH3)4 ion hydrolyzes to CuII(OH)(NH3)3 ion to gain redox activity. The CuII(OH)(NH3)3 ion also transfers between neighboring zeolite cages to form highly reactive reaction intermediates.

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Interplay between copper redox and transfer and support acidity and topology in low temperature NH3-SCR - Nature Communications

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Interplay between copper redox and transfer and support acidity and topology in low temperature NH3-SCR - Nature Communications

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