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Enhanced CO2 utilization in dry reforming of methane achieved through nickel-mediated hydrogen spillover in zeolite crystals - Nature Catalysis
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Transformation of CO2 into precursors for chemicals and fuels by self-contained reducing gas contaminants (for example, CH4) is attractive from a carbon economy perspective. Reducing as much CO2 as possible using a limited amount of reducing gas would be ideal, but general dry reforming (DRM) schemes consume stoichiometric amounts of methane for CO2 reduction. Here we develop a process with high reducibility of methane relative to conventional DRM, using up to 2.9 mol of CO2 per mol of CH4.
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