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Exploration of the bio-analogous asymmetric C–C coupling mechanism in tandem CO2 electroreduction - Nature Catalysis
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C–C coupling is a critical step of CO2 fixation in constructing the carbon skeleton of value-added multicarbon products. The Wood–Ljungdahl pathway is an efficient natural process through which microbes transform CO2 into methyl and carbonyl groups and subsequently couple them together. This asymmetric coupling mechanism remains largely unexplored in inorganic CO2 electroreduction.
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